Bali became a star in the 1950s. She had also worked earlier with her future brother-in-law Raj Kapoor in Bawre Nain and with her future father-in-law Prithviraj Kapoor in Anand Math. Unlike other actresses who gave up films after marrying into the Kapoor family, Bali kept acting until her death.
Her secretary was Surinder Kapoor, father of producer Boney Kapoor and actor Anil Kapoor.